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Supercooled fogs can have an important radiative impact at the surface of the Greenland Ice Sheet, but they are difficult to detect and our understanding of the factors that control their lifetime and radiative properties is limited by a lack of observations. This study demonstrates that spectrally resolved measurements of downwelling longwave radiation can be used to generate retrievals of fog microphysical properties (phase and particle effective radius) when the fog visible optical depth is greater than ∼0.25. For 12 cases of fog under otherwise clear skies between June and September 2019 at Summit Station in central Greenland, nine cases were mixed‐phase. The mean ice particle (optically‐equivalent sphere) effective radius was 24.0 ± 7.8 µm, and the mean liquid droplet effective radius was 14.0 ± 2.7 µm. These results, combined with measurements of aerosol particle number concentrations, provide evidence supporting the hypotheses that (a) low surface aerosol particle number concentrations can limit fog liquid water path, (b) fog can act to increase near‐surface aerosol particle number concentrations through enhanced mixing, and (c) multiple fog events in quiescent periods gradually deplete near‐surface aerosol particle number concentrations.

 

Abstract. This study presents the first full annual cycle (2019–2020) of ambient surface aerosol particle number concentration measurements (condensationnuclei > 20 nm, N20) collected at Summit Station (Summit), in the centre of the Greenland Ice Sheet (72.58∘ N, −38.45∘ E; 3250 ma.s.l.). The mean surface concentration in 2019 was 129 cm−3, with the 6 h mean ranging between 1 and 1441 cm−3. The highest monthly mean concentrations occurred during the late spring and summer, with the minimum concentrations occurring in February (mean: 18 cm−3). High-N20 events are linked to anomalous anticyclonic circulation over Greenland and the descent of free-tropospheric aerosol down to the surface, whereas low-N20 events are linked to anomalous cyclonic circulation over south-east Greenland that drives upslope flow and enhances precipitation en route to Summit. Fog strongly affects particle number concentrations, on average reducing N20 by 20 % during the first 3 h of fog formation. Extremely-low-N20 events (< 10 cm−3) occur in all seasons, and we suggest that fog, and potentially cloud formation, can be limited by low aerosol particle concentrations over central Greenland. 

Decreases in stratospheric NO_xassociated with enhanced aerosol have been observed after large volcanic eruptions, for example, after the eruption of Mount Pinatubo in 1991. While the 1991 Mount Pinatubo eruption was the last large explosive eruption, recent studies have shed light on the impacts of moderate‐sized eruptions since the year 2000 on the global stratospheric aerosol budget. We use an ensemble of simulations from a coupled climate‐chemistry model to quantify and analyze changes in NO and NO₂(NO_x), N₂O₅, HNO₃, ClO, and ClONO₂during periods of increased stratospheric volcanic aerosol concentrations since 2000. By using an ensemble approach, we are able to distinguish forced responses from internal variability. We also compare the model ensemble results to satellite measurements of these changes in atmospheric composition, including measurements from the Optical Spectrograph and Infrared Imaging Spectrometer on the Odin satellite and the Aura Microwave Limb Sounder. We find decreases in stratospheric NO_xconcentrations up to 20 hPa, consistent with increases in stratospheric HNO₃concentrations. The HNO₃perturbations also extend higher, up to 5 hPa, associated with periods of increased volcanic aerosol concentrations in both model simulations and observations, though correlations with volcanic aerosol are considerably higher in the model simulations. The model simulates increases in ClO at altitudes and magnitudes similar to the NO_xreductions, but this response is below the detectable limit in the available observations (100 pptv). We also demonstrate the value of accounting for transport‐related anomalies of atmospheric trace gases by regression onto N₂O anomalies.

 

Ice crystals commonly adopt a horizontal orientation under certain aerodynamic and electrodynamic conditions that occur in the atmosphere. While the radiative impact of horizontally oriented ice crystals (HOIC) has been theoretically studied with respect to their impact on shortwave cloud albedo, the longwave impact remains unexplored. This work analyzes the occurrence of HOIC at Summit, Greenland, from July 2015 to June 2017. Using polarization lidar and ancillary atmospheric sensors, ice crystal orientations are identified and used to interpret cloud radiative impact on the surface radiation budget. We find HOIC occur in at least 25.6% of all ice‐only column observations. We find that the shortwave impact of HOIC is to increase cloud radiative effect by approximately 22% for a given solar zenith angle. We also find that the longwave impact of HOIC compared to randomly oriented ice crystals are statistically different at the p < 0.01 significance level, increasing the surface radiative effect by approximately 8% for clouds with infrared optical depths < ~1. We suggest that the observed difference between the surface radiative effect for clouds containing randomly oriented ice crystals and HOIC may be due to enhanced scattering, but this hypothesis needs to be further explored with more detailed observations and modeling.